Magnetic, electrical and thermodynamic properties of RE8Pd24In
Identifieur interne : 003D43 ( Main/Repository ); précédent : 003D42; suivant : 003D44Magnetic, electrical and thermodynamic properties of RE8Pd24In
Auteurs : RBID : Pascal:11-0006829Descripteurs français
- Pascal (Inist)
- Loi Curie Weiss, Propriété thermodynamique, Phénomène transport, Diffraction RX, Conductivité électrique, Susceptibilité magnétique, Aimantation, Chaleur massique, Antiferromagnétisme, Lanthanide alliage, Transition magnétique, Paramètre cristallin, Palladium alliage, Indium alliage, Alliage ternaire, Réseau cubique.
English descriptors
- KwdEn :
Abstract
Investigations of magnetic, transport and thermodynamic properties of RE8Pd24In (RE = Pr, Nd, Gd, Tb, Dy, Ho, Er and Tm) are reported through measurements of X-ray diffraction, electrical resistivity (ρ(T)), magnetic susceptibility (χ(T)), magnetization (σ(μ0H)) and heat capacity (Cp(T)). These ternary compounds have the cubic AuCu3-type structure. Compounds with RE = Gd and Tb order antiferromagnetically (AF) and exhibit magnetic transitions observed in their χ (T) and Cp(T). ρ(T) results for the Gd and Tb compounds indicate a minimum above the magnetic phase transition temperature TN, and an increase in ρ(T) upon further cooling as a precursor ofAF order at lower temperatures. χ (T) data at high temperatures follow the Curie-Weiss relation for all compounds and give effective moment values close to those expected for the free RE3+-ion. Enhanced values of the electronic contribution to the heat capacity were observed for Gd8Pd24In and Tb8Pd24In.
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Pd<sub>24</sub>
In</title>
<author><name sortKey="Tchoula Tchokonte, M B" uniqKey="Tchoula Tchokonte M">M. B. Tchoula Tchokonte</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Physics, University of the Western Cape, Private BagX 17</s1>
<s2>Bellville 7535</s2>
<s3>ZAF</s3>
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<country>Afrique du Sud</country>
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<author><name sortKey="Du Plessis, P De V" uniqKey="Du Plessis P">P. De V. Du Plessis</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Department of Physics, University of Johannesburg, PO Box 524</s1>
<s2>Auckland Park 2006</s2>
<s3>ZAF</s3>
<sZ>2 aut.</sZ>
<sZ>4 aut.</sZ>
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<country>Afrique du Sud</country>
<wicri:noRegion>Auckland Park 2006</wicri:noRegion>
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<affiliation wicri:level="4"><inist:fA14 i1="03"><s1>School of Physics, University of the Witwatersrand, Private Bag 3, PO Wits 2050</s1>
<s2>Johannesburg</s2>
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<sZ>2 aut.</sZ>
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<author><name sortKey="Kaczorowski, D" uniqKey="Kaczorowski D">D. Kaczorowski</name>
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<author><name sortKey="Strydom, A M" uniqKey="Strydom A">A. M. Strydom</name>
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<term>Aimantation</term>
<term>Chaleur massique</term>
<term>Antiferromagnétisme</term>
<term>Lanthanide alliage</term>
<term>Transition magnétique</term>
<term>Paramètre cristallin</term>
<term>Palladium alliage</term>
<term>Indium alliage</term>
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<front><div type="abstract" xml:lang="en">Investigations of magnetic, transport and thermodynamic properties of RE<sub>8</sub>
Pd<sub>24</sub>
In (RE = Pr, Nd, Gd, Tb, Dy, Ho, Er and Tm) are reported through measurements of X-ray diffraction, electrical resistivity (ρ(T)), magnetic susceptibility (χ(T)), magnetization (σ(μ<sub>0</sub>
H)) and heat capacity (C<sub>p</sub>
(T)). These ternary compounds have the cubic AuCu<sub>3</sub>
-type structure. Compounds with RE = Gd and Tb order antiferromagnetically (AF) and exhibit magnetic transitions observed in their χ (T) and C<sub>p</sub>
(T). ρ(T) results for the Gd and Tb compounds indicate a minimum above the magnetic phase transition temperature T<sub>N</sub>
, and an increase in ρ(T) upon further cooling as a precursor ofAF order at lower temperatures. χ (T) data at high temperatures follow the Curie-Weiss relation for all compounds and give effective moment values close to those expected for the free RE<sup>3+</sup>
-ion. Enhanced values of the electronic contribution to the heat capacity were observed for Gd<sub>8</sub>
Pd<sub>24</sub>
In and Tb<sub>8</sub>
Pd<sub>24</sub>
In.</div>
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<sZ>4 aut.</sZ>
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Pd<sub>24</sub>
In (RE = Pr, Nd, Gd, Tb, Dy, Ho, Er and Tm) are reported through measurements of X-ray diffraction, electrical resistivity (ρ(T)), magnetic susceptibility (χ(T)), magnetization (σ(μ<sub>0</sub>
H)) and heat capacity (C<sub>p</sub>
(T)). These ternary compounds have the cubic AuCu<sub>3</sub>
-type structure. Compounds with RE = Gd and Tb order antiferromagnetically (AF) and exhibit magnetic transitions observed in their χ (T) and C<sub>p</sub>
(T). ρ(T) results for the Gd and Tb compounds indicate a minimum above the magnetic phase transition temperature T<sub>N</sub>
, and an increase in ρ(T) upon further cooling as a precursor ofAF order at lower temperatures. χ (T) data at high temperatures follow the Curie-Weiss relation for all compounds and give effective moment values close to those expected for the free RE<sup>3+</sup>
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